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  • Differentiating ion transport of water-in-salt electrolytes within . . .
    Several research groups have reported the ion dynamics in bulk water-in-salt electrolytes of LiTFSI using PFG-NMR 15–18 † They were used to quantify the non-ideality in the water-in-salt electrolytes from the ratio in eqn (4) This indicates the degree of ion dissociation or ionicity, which is also known as the inverse Haven ratio
  • Mobility-viscosity decoupling and cation transport in water-in-salt . . .
    The physicochemical properties of WiS electrolytes are not yet completely understood Using a wide variety of techniques, such as FT-IR and Raman spectroscopy, Small Angle Neutron Scattering (SANS), and Molecular Dynamics (MD), Borodin et al [13] have proposed the formation of nano-heterogeneities in 21 mol kg −1 LiTFSI aqueous solution, in the shape of interpenetrating dynamic nano-domains
  • Water-In-Salt LiTFSI Aqueous Electrolytes (2): Transport Properties and . . .
    At high salt concentrations of 20 m, the calculated viscosity, self-diffusion coefficients, ionic conductivity, the inverse Haven ratio, and the Li + apparent transference number all agree with previous experimental results quantitatively
  • Li+ hopping mechanism in LiTFSI water-in-salt electrolyte identified by . . .
    The high Li+ apparent transference number in the LiTFSI water-in-salt electrolyte was captured by MD simulations and the dominant Li+ conduction mechanism in the highly concentrated LiTFSI water-in-salt electrolyte was identified to be hopping between water and TFSI- anions Significance and Impact
  • Water-In-Salt LiTFSI Aqueous Electrolytes (2): Transport Properties and . . .
    At high salt concentrations of 20 m, the calculated viscosity, self-diffusion coefficients, ionic conductivity, the inverse Haven ratio, and the Li+ apparent transference number all agree with previous experimental results quantitatively Furthermore, analyses show that the high apparent transference number for Li+ i
  • Effect of salt concentration in aqueous LiTFSI electrolytes on the . . .
    The enhancement of the electrolyte stability window and cell potential in water-in-LiTFSI electrolyte when using stainless steel [4, 11] and aluminum [12] electrodes is generally attributed to the negligible amount of free water, owing to the low water-to-salt ratio, that causes nearly all water molecules to be involved in solvating Li + ions [13, 14]
  • The hydrotropic effect of ionic liquids in water‐in‐salt electrolytes
    compares this ratio for selected LiTFSI–RTIL–water hybrid electrolytes with that of 21m LiTFSI The number of available water molecules per lithium ion shrinks from 2 65 in 21m LiTFSI to 1 39 in a solution containing 40m LiTFSI and 20m RTIL (sample 40 20) Pushing the LiTFSI content to its solubility limit reduces the ratio further to 1 23
  • Ion transport in semi-solid in-salt electrolytes: LiTFSI–H
    The water-in-salt (WIS) electrolyte represents a newly developed battery electrolyte system with high ionic conductivity that enables cells with a broader electrochemical window and improved cyclability Several theories have been proposed to explain the co-existence of high conductivity and salt concentrati 2023 Journal of Materials Chemistry A HOT Papers
  • Effect of Salt Concentration in Water-In-Salt Electrolyte on . . .
    Effect of Salt Concentration in Water-In-Salt Electrolyte on Supercapacitor Applications Imgon Hwang, (LiTFSI) electrolyte, revealing a high specific capacitance despite its elevated viscosity and restricted ionic conductivity Our approach integrated resonance intensities with a Gaussian-to-Lorentzian ratio Wiley VCH Dienstag, 14 05
  • Water-In-Salt LiTFSI Aqueous Electrolytes (2): Transport Properties and . . .
    The transport properties of water-in-salt lithium bis­(trifluoromethane sulfonyl)­imide (LiTFSI) aqueous electrolytes were studied using classical molecular dynamics (MD) simulations At high salt concentrations of 20 m, the calculated viscosity, self-diffusion coefficients, ionic conductivity, the inverse Haven ratio, and the Li+ apparent transference number all agree with previous
  • Design strategies and research progress for Water-in-Salt electrolytes . . .
    The co-solvents WIS electrolyte (also called localized Water-in-Salt electrolyte or bisolvent-in-salt) is a composite electrolyte with two or more liquid phases composed of WIS electrolyte and additional organic solvents (BSiS-A 0 5) by further regulating the content of H 2 O molecules (LiTFSI H 2 O ACN molar ratio = 1:1 11:1 11) [196
  • Water-In-Salt LiTFSI Aqueous Electrolytes (2): Transport . . . - scite
    Supporting: 3, Contrasting: 1, Mentioning: 31 - The transport properties of water-in-salt lithium bis­(trifluoromethane sulfonyl)­imide (LiTFSI) aqueous electrolytes were studied using classical molecular dynamics (MD) simulations At high salt concentrations of 20 m, the calculated viscosity, self-diffusion coefficients, ionic conductivity, the inverse Haven ratio, and the Li+ apparent





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